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    Frenkel line and solubility maximum in supercritical fluids. 
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    Frenkel line and solubility maximum in supercritical fluids.

    Volume
    91
    Pagination
    012112 - ?
    DOI
    10.1103/PhysRevE.91.012112
    Journal
    Phys Rev E Stat Nonlin Soft Matter Phys
    Issue
    1
    Metadata
    Show full item record
    Abstract
    A new dynamic line, the Frenkel line, has recently been proposed to separate the supercritical state into rigid-liquid and nonrigid gaslike fluid. The location of the Frenkel line on the phase diagram is unknown for real fluids. Here we map the Frenkel line for three important systems: CO(2), H(2)O, and CH(4). This provides an important demarcation on the phase diagram of these systems, the demarcation that separates two distinct physical states with liquidlike and gaslike properties. We find that the Frenkel line can have a similar trend as the melting line above the critical pressure. Moreover, we discuss the relationship between unexplained solubility maxima and Frenkel line, and we propose that the Frenkel line corresponds to the optimal conditions for solubility.
    Authors
    Yang, C; Brazhkin, VV; Dove, MT; Trachenko, K
    URI
    http://qmro.qmul.ac.uk/xmlui/handle/123456789/7123
    Collections
    • Physics and Astronomy [1176]
    Language
    eng
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